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First make sure the webservers and application servers can communicate with each other by open firewall rules, if not done yet.
Set the default local nodes to user authenticate and make sure the node are pingable from the other environment.
After this set the remote nodes to be trusted and SSO of PeopleSoft is done.
Read more in detail in PeopleBooks.
PeopleBooks > PeopleTools 8.52: Security Administration > Implementing Single Signon > Implementing PeopleSoft-Only Single Signon